Atmospheric Chemistry & Modeling (ACM) Group, Peking University

journal · 2022

Considerable unaccounted local sources of NOx emissions in China revealed from satellite

Kong, H., Lin, J.-T. *, Chen, L.-L., Zhang, Y.-H., Yan, Y.-Y., Liu, M.-Y., Ni, R.-J., Liu, Z., and Weng, H.-J.

Environmental Science & Technology, 56, 7131–7142

Abstract

High-resolution (e.g., 5 km) emission data of nitrogen oxides (NO x =N O+N O 2) provide localized knowledge of pollution sources for targeted regulations, yet such data are lacking or inaccurate over most regions at present. Here we improve our PHLET-based inversion method to derive NO x emissions in China at a 5-km resolution in summer 2019, based on the TROPOMI-POMINO satellite product of nitrogen dioxide (NO 2) columns. With low computational costs, our inversion explicitly accounts for the e ffects of horizontal transport and nonlinear chemistry. We find numerous small-to-medium sources related to minor roads and small human settlements at relatively low a ffluence levels, in addition to clear emission signals along major transportation lines, consistent with road line density and Tencent location data. Many smallto-medium sources and transportation emissions are unclear or missing in the spatial distributions of four widely used emission inventories. Our emissions o ffer a unique reference for targeted emission control.

Keywords

  • NOx emission
  • high resolution
  • satellite
  • China
  • TROPOMI
  • ■ INTRODUCTION
  • short-lived air pollutant. A t present
  • place
  • high-resolution (i.e

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